Umm, no, that really won't work in the way you may be thinking. Differential quenches/hardening are the result of the formation of pearlite at the spine and martensite at the edge. In this case, the softer phase (pearlite) is the most stable phase possible in an iron-carbon system. D-2 cannot make pearlite, this is what makes it air hardening. So, what you will get is still martensite, but it will be mixed with austenite- literally one of the most unstable phases you can have. Yes, you will gain some toughness, but it will be because you have not completed the hardening process and should you get conversion of the metastable austenite later on it can be an issue in several ways.